Metal Doped Core-Shell Metal-Organic Frameworks@Covalent Organic Frameworks (MOFs@COFs) Hybrids as a Novel Photocatalytic Platform
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- Title
- Metal Doped Core-Shell Metal-Organic Frameworks@Covalent Organic Frameworks (MOFs@COFs) Hybrids as a Novel Photocatalytic Platform
- Authors
- Sun, Dengrong; Jang, Seungwook; Yim, Se-Jun; Ye, Lin; Kim, Dong-Pyo
- Date Issued
- 2018-03
- Publisher
- WILEY-V C H VERLAG GMBH
- Abstract
- Metal doped core-shell Metal-Organic Frameworks@Covalent Organic Frameworks (MOFs@COFs) are presented as a novel platform for photocatalysis. A palladium (Pd) doped MOFs@COFs in the form of Pd/TiATA@LZU1 shows excellent photocatalytic performance for tandem dehydrogenation and hydrogenation reactions in a continuous-flow microreactor and a batch system, indicating the great potential of the metal doped MOFs@COFs as a multifunctional platform for photocatalysis. Explanations for the performance enhancement are elucidated. An integrated dual-chamber microreactor coupled with the metal doped MOFs@COFs is introduced to demonstrate a concept of an intensified green photochemical process, which can be broadly extended to challenging liquid-gas tandem and cascade reactions.
- URI
- https://oasis.postech.ac.kr/handle/2014.oak/96050
- DOI
- 10.1002/adfm.201707110
- ISSN
- 1616-301X
- Article Type
- Article
- Citation
- ADVANCED FUNCTIONAL MATERIALS, vol. 28, no. 13, page. 1707110, 2018-03
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