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Operando Stability of Single‐Atom Electrocatalysts SCIE SCOPUS

Title
Operando Stability of Single‐Atom Electrocatalysts
Authors
Bae, GeunsuHan, SunghoonOh, Hyung-SukChoi, Chang Hyuck
Date Issued
2023-01
Publisher
John Wiley & Sons Ltd.
Abstract
Single-atom catalysts (SACs) are appealing next-generation catalysts for various electrochemical technologies. Along with significant breakthroughs in their initial activity, SACs now face the next challenge for their viable applications, insufficient operational stability. In this Minireview, we summarize the current knowledge of SAC degradation mechanisms mainly based on Fe-N-C SACs, some of the most investigated SACs. Recent studies on isolated metal, ligand, and support degradations are introduced, and the underlying fundamentals of each degradation path are categorized into active site density (SD) and turnover frequency (TOF) losses. Finally, we discuss the challenges and prospects for the future outlook of stable SACs.
URI
https://oasis.postech.ac.kr/handle/2014.oak/115611
DOI
10.1002/anie.202219227
ISSN
1433-7851
Article Type
Article
Citation
Angewandte Chemie - International Edition, 2023-01
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