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Dopant impact on the activity and thermostability of Ni-Mg/Al2O3 catalyst for SNG reaction

Title
Dopant impact on the activity and thermostability of Ni-Mg/Al2O3 catalyst for SNG reaction
Authors
Yan Xiang
Date Issued
2013
Publisher
포항공과대학교
Abstract
In order to improve Ni-Mg/Al2O3 catalyst activity and thermostability for SNG reaction, several dopants(La, Ce, Ca, Fe, Co, Mn, Sr, Zr) were applied to investigate their performance under harsh ageing environment. Impregnation was used to load dopant. Characterization analysis(XRD, TPR, BET, TGA and TEM) were applied to explore the properties of reduced and used catalysts. Among the dopants, La is a promising additive for its high initial activity and excellent thermostability. Other additives doped catalysts exhibited gradual activity loss during the ageing period. La additive helps to stabilize metallic nickel phase through the formation of LaAlO3 which is observed in the XRD pattern. By changing the amount of La, we compared their performance. Among the catalysts tested, 5wt% La exhibits the best performance for improving the activity and thermostability of Ni-Mg/Al2O3 catalyst.
URI
http://postech.dcollection.net/jsp/common/DcLoOrgPer.jsp?sItemId=000001560276
http://oasis.postech.ac.kr/handle/2014.oak/1844
Article Type
Thesis
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